Example: Numerical Frequencies, spin-orbit coupled ZORA: UF6¶
#! /bin/sh
# Summary:
# - Geometry optimization
# - Frequencies with symmetric displacements
# - Both for scalar relativistic ZORA and spin-orbit coupled ZORA
# == Geometry optimization ==
# Here only the spin-orbit coupled input file for ADF is given (in the scalar
# relativistic case change 'spinorbit' in 'scalar'). The resulting TAPE21 is
# saved such that it can be used in the frequency calculation.
$ADFBIN/adf <<eor
Title UF6 geometry optimization: scalar ZORA
BeckeGrid
Quality good
End
Geometry
converge grad=1e-4
End
relativistic scalar zora
Basis
Type TZP
end
ATOMS
1 U 0.00000 0.00000 0.00000
2 F 2.00000 0.00000 0.00000
3 F -2.00000 0.00000 0.00000
4 F 0.00000 2.00000 0.00000
5 F 0.00000 -2.00000 0.00000
6 F 0.00000 0.00000 2.00000
7 F 0.00000 0.00000 -2.00000
END
eor
mv TAPE21 UF6.t21
# == Frequencies with symmetric displacements ==
# Computation of frequencies by symmetric displacements. The assumed equilibrium
# input structure should be given in Cartesian coordinates. The calculation
# starts with the optimized structure read from UF6.t21 (restart file). Again
# only the spin-orbit coupled input file for ADF is given.
# The symmetry is determined automatically by the program as O(H), from the
# input coordinates. During the calculation first symmetric atomic displacements
# are constructed. The number of such displacements in each irreducible
# representation corresponds to the number of frequencies with the corresponding
# symmetry. All displaced geometries within one representation have the same
# symmetry, which enables us to use it to speed up the computation
# significantly.
$ADFBIN/adf <<eor
Title UF6 frequencies and IR intensities: scalar ZORA
Restart
File UF6.t21
End
Geometry
Frequencies Symm=True
End
BeckeGrid
Quality good
End
relativistic scalar zora
Fragments
U t21.U
F t21.F
end
ATOMS
1 U 0.00000 0.00000 0.00000
2 F 2.00000 0.00000 0.00000
3 F -2.00000 0.00000 0.00000
4 F 0.00000 2.00000 0.00000
5 F 0.00000 -2.00000 0.00000
6 F 0.00000 0.00000 2.00000
7 F 0.00000 0.00000 -2.00000
END
eor
rm TAPE21 logfile UF6.t21
# Optimization and frequencies for spinorbit ZORA
$ADFBIN/adf <<eor
Title UF6 geometry optimization: spinorbit ZORA
BeckeGrid
Quality good
End
Geometry
converge grad=1e-4
End
relativistic spinorbit zora
Fragments
U t21.U
F t21.F
end
ATOMS
1 U 0.00000 0.00000 0.00000
2 F 2.00000 0.00000 0.00000
3 F -2.00000 0.00000 0.00000
4 F 0.00000 2.00000 0.00000
5 F 0.00000 -2.00000 0.00000
6 F 0.00000 0.00000 2.00000
7 F 0.00000 0.00000 -2.00000
END
eor
mv TAPE21 UF6.t21
$ADFBIN/adf <<eor
Title UF6 frequencies and IR intensities: spinorbit ZORA
Restart
File UF6.t21
End
Geometry
Frequencies Symm=True
End
BeckeGrid
Quality good
End
relativistic spinorbit zora
Fragments
U t21.U
F t21.F
end
ATOMS
1 U 0.00000 0.00000 0.00000
2 F 2.00000 0.00000 0.00000
3 F -2.00000 0.00000 0.00000
4 F 0.00000 2.00000 0.00000
5 F 0.00000 -2.00000 0.00000
6 F 0.00000 0.00000 2.00000
7 F 0.00000 0.00000 -2.00000
END
eor
rm TAPE21 logfile UF6.t21