Example: NOCV: CH2 – Cr(CO)5¶
#! /bin/sh
# Example for calculation of ETS-NOCV for spin-restricted fragments. ETS-NOCV:
# energy analysis using the Natural Orbitals for Chemical Valence. The CH2
# molecule and Cr(CO)5 are the fragments, which form Cr(CO)5 CH2 molecule.
# First the two fragments are calculated.
AMS_JOBNAME=CH2 $AMSBIN/ams <<eor
System
atoms
C -0.429104 1.732058 -0.225052
H 0.407023 2.440417 -0.352323
H -1.385325 2.281354 -0.254124
end
end
Task SinglePoint
Engine ADF
title CrCO5--[CH2] run from CrCO5 and CH2 closed shell fragments,FULL electron calc.!
basis
core None
type DZP
end
symmetry NOSYM
xc
gga becke perdew
end
EndEngine
eor
AMS_JOBNAME=CrCO5 $AMSBIN/ams <<eor
System
atoms
Cr -0.248053 -0.169062 0.005810
C -0.072963 -2.080685 0.229583
O 0.030811 -3.223220 0.361925
C -0.182894 0.049840 1.909128
O -0.142780 0.212309 3.050403
C -0.299940 -0.409118 -1.894730
O -0.331795 -0.521589 -3.042336
C -2.138631 -0.242152 0.075713
O -3.295036 -0.249916 0.115045
C 1.624487 0.092244 -0.083118
O 2.763411 0.288575 -0.140976
end
end
Task SinglePoint
Engine ADF
title [CrCO5] run
basis
Type DZP
Core None
PerAtomType Symbol=Cr Type=TZP
end
symmetry NOSYM
xc
gga becke perdew
end
EndEngine
eor
# Next these fragments are used in the calculation of the full complex. The keys
# ETSNOCV and 'PRINT etslowdin' are needed in this case to to analyze the
# bonding in the molecule with respect to the fragments. The symmetry must be
# NOSYM.
AMS_JOBNAME=CrCO5_CH2 $AMSBIN/ams <<eor
System
atoms
C -0.429104 1.732058 -0.225052 adf.f=f1
Cr -0.248053 -0.169062 0.005810 adf.f=f2
C -0.072963 -2.080685 0.229583 adf.f=f2
O 0.030811 -3.223220 0.361925 adf.f=f2
C -0.182894 0.049840 1.909128 adf.f=f2
O -0.142780 0.212309 3.050403 adf.f=f2
C -0.299940 -0.409118 -1.894730 adf.f=f2
O -0.331795 -0.521589 -3.042336 adf.f=f2
C -2.138631 -0.242152 0.075713 adf.f=f2
O -3.295036 -0.249916 0.115045 adf.f=f2
C 1.624487 0.092244 -0.083118 adf.f=f2
O 2.763411 0.288575 -0.140976 adf.f=f2
H 0.407023 2.440417 -0.352323 adf.f=f1
H -1.385325 2.281354 -0.254124 adf.f=f1
end
end
Task SinglePoint
Engine ADF
title CrCO5--[CH2], etsnocv acitivated by etsnocv and print etslowdin
etsnocv
ekmin 1.5
enocv 0.05
rhokmin 1.e-3
end
fragments
f1 CH2.results/adf.rkf
f2 CrCO5.results/adf.rkf
end
print etslowdin
symmetry NOSYM
xc
gga becke perdew
end
EndEngine
eor